The paint sounds promising. It just needs to stick to ASA. I’m not sanding anything either so it’s not flat but that might be a good thing to increase surface area for the paint to bind to.
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Trees are inefficient too but we actually already know what we need to do to ramp up the efficiency of the photosynthesis process in trees with genetic tinkering.
The bigger problem is that we have reached a point where trees aren’t enough anymore. The oceans have acidified. There’s just too much co2 to capture at this point.